Weining Man

Princeton University

Geometry and Symmetry in Experimental Condensed Matter Physics and Material Science

Photonic Quasicrystals & Random Ellipsoid Packings

Friday, February 22, 2008, 4:00 p.m.
Refreshments at 3:45 p.m.

ABSTRACT

Geometry and symmetry play an important role in the design of new materials. In particular this talk investigates photonic quasicrystals and ellipsoid packings, problems in which the geometry of the building blocks and the structural symmetry determine the physical properties. Photonic quasicrystals are constructed from dielectric material arranged in a quasiperiodic pattern whose rotational symmetry is forbidden for periodic crystals. Because quasicrystals have higher point group symmetry than ordinary crystals, they can have more uniform bandgaps. Since calculating the band structure of 3D photonic quasicrystals is fundamentally challenging, and to date beyond the range of computation in a reasonable time, we decided to answer the question experimentally. We constructed the world's first and largest (in terms of the number of units) 3D icosahedral Photonic quasicrystal (composed of polymer) using stereolithography. With our novel method to make polar plots of its microwave transmission vs. frequency and incident angle, we obtained the first-ever visualization of the Brillouin zone of a quasicrystal. Before our experimental work it was not at all clear that Brillouin zones existed or had physical meaning in quasicryatals. We proved that the nearly spherical Brillouin zones of 3D icosahedral quasicrystals make them one of the most promising candidates for complete photonic bandgaps found to date. For ellipsoidal granular material packing, we designed and performed different experiments, including MRI scans, to extrapolate the bulk density of an infinitely large random system, using a limited number of particles. We found in both experiments and simulations that ellipsoids can pack randomly more densely than spheres because of their extra degree of freedom associated with their rotational axes. Surprisingly the packing fraction has a cusp-like minimum for spheres and increases sharply with aspect ratios different from unity. A major fundamental question remains as to whether any shape particle can produce an amorphous packing of higher density than its crystalline packing. It will be enlightening to find the correlations between this ratio of amorphous and crystal packings and features of the equilibrium phase diagrams for various particle shapes.